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• W2532928369 abstract "Abstract In this study, the kinetics of glycerol pyrolysis over a 3wt%Pr-20wt%Ni/77wt%α-Al 2 O 3 catalyst was investigated. The catalyst was synthesized via wet-impregnation method and was characterized using temperature-programmed calcination (TPC), temperature-programmed reduction (TPR), N 2 -physisorption, FESEM imaging, X-ray diffraction and CO 2 -/NH 3 -temperature-programmed desorption (TPD). The catalytic activity of the as-synthesized 3 wt% Pr-Ni/α-Al 2 O 3 catalyst was evaluated in a stainless steel fixed bed reactor at temperatures that ranged from 973 K to 1073 K and a weight-hourly-space-velocity (WHSV) of 4.5 × 10 4  ml g −1  h −1 under the atmospheric condition. The main gaseous products from catalytic glycerol pyrolysis were H 2 , CO, CO 2 and CH 4 (descending ranking) with the highest H 2 formation rate and H 2 yield of 0.02593 mol g cat −1  s −1 and 29.04%, respectively. The analysis of the kinetic data obtained from the glycerol pyrolysis showed activation energy of 37.36 kJ mol −1 . Based on the mechanistic modeling, it can be deduced that the rate determining step of the glycerol pyrolysis was via a single site associative adsorption with molecular surface reaction as the rate-determining step." @default.
• W2532928369 created "2016-10-28" @default.
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• W2532928369 date "2017-02-01" @default.
• W2532928369 modified "2023-09-24" @default.
• W2532928369 title "Renewable syngas production from thermal cracking of glycerol over praseodymium-promoted Ni/Al 2 O 3 catalyst" @default.
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• W2532928369 doi "https://doi.org/10.1016/j.applthermaleng.2016.10.126" @default.
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