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- W2533484599 abstract "Monte Carlo track chemistry simulations of the low linear energy transfer radiolysis of pure, deaerated liquid water have been used in combination with a spherical spur model to examine the effect of temperature on the in situ formation of H3O+ ions and the corresponding abrupt transient “acid-spike” response that is observed after irradiation. The magnitude and duration of this acid-spike effect were found to be a very sensitive function of temperature. At 25 °C, it is most intense at times less than ∼1 ns, with a pH of 3.3 remaining nearly constant. In contrast, at higher temperatures, there is an increasingly acidic but much shorter pH response. At 350 °C, the pH is around 1.7 on a time scale of ∼10 ps. At longer times, the pH gradually increases for all temperatures, ultimately reaching a constant value corresponding to the non-radiolytic, pre-irradiation concentration of H3O+ arising through water’s autoprotolysis at ∼1–10 μs following irradiation. It does not appear that this transient acid-spike ef..." @default.
- W2533484599 created "2016-10-28" @default.
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- W2533484599 date "2016-10-25" @default.
- W2533484599 modified "2023-10-18" @default.
- W2533484599 title "GENERATION OF ULTRAFAST TRANSIENT ACID SPIKES IN HIGH-TEMPERATURE WATER IRRADIATED WITH LOW LINEAR ENERGY TRANSFER RADIATION" @default.
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- W2533484599 doi "https://doi.org/10.12943/cnr.2016.00013" @default.
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