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- W2534771223 abstract "Molybdenum carbide on sulfated zirconia was prepared by impregnation of MoO3 on sulfated zirconia to give a loading of 5 wt% followed by carburisation at 923 K in a mixture of CH4/H2 (4:1). The resulting catalyst was characterised by N2 adsorption–desorption, CO chemisorption, FTIR of pyridine adsorption, XRD, TPR, TGA, Raman and SEM–EDX. This combination of characterisation studies suggests formation of a well-dispersed Mo2C phase over tetragonal zirconia. When employed in the hydroconversion of n-heptane, high temperature and low space velocity lead to substantial cracking. However, under some conditions, an increase in the research octane number (RON) from 0 (n-heptane) to ca. 50 was attained. Between 723 and 873 K, n-heptane is mainly cracked to iso-pentane and ethane. The product distribution as a function of conversion suggests that the reaction did not simply follow a consecutive reaction pathway, but that other parallel routes were involved." @default.
- W2534771223 created "2016-10-28" @default.
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- W2534771223 date "2016-10-19" @default.
- W2534771223 modified "2023-10-01" @default.
- W2534771223 title "n-Heptane hydroconversion over sulfated-zirconia-supported molybdenum carbide catalysts" @default.
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- W2534771223 doi "https://doi.org/10.1007/s13203-016-0172-z" @default.
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