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- W2535263117 abstract "We report the exfoliation of graphite and simultaneous N doping of graphene by two methods: supercritical ammonia treatment and liquid-phase exfoliation with NH4OH. While the supercritical ammonia allowed N doping at a level of 6.4 atom % in 2 h, the liquid-phase exfoliation with NH4OH allowed N doping at a level of 2.7 atom % in 6 h. The N doped graphene obtained via the supercritical ammonia route had few layers (<5) and showed large lateral flake size (∼8 μm) and low defect density (ID/IG < 0.6) in spite of their high level of N doping. This work is the first demonstration of supercritical ammonia as an exfoliation agent and N doping precursor for graphene. Notably, the N doped graphene showed electrocatalytic activity toward oxygen reduction reaction with high durability and good methanol tolerance compared to those of commercial Pt/C catalyst." @default.
- W2535263117 created "2016-10-28" @default.
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- W2535263117 date "2016-11-03" @default.
- W2535263117 modified "2023-10-09" @default.
- W2535263117 title "Simultaneous Graphite Exfoliation and N Doping in Supercritical Ammonia" @default.
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- W2535263117 doi "https://doi.org/10.1021/acsami.6b10570" @default.
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