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• W2535303503 abstract "ABSTRACT A series of dinuclear Dy III acetate complexes containing three different hydrazine‐functionalized Schiff‐base ligands ( hmb , hmi, and hb ) have been synthesized by one‐pot reaction with Dy(OAc) 3 ·4H 2 O as the metal precursor. [Dy 2 ( hmb ) 2 (OAc) 4 ]·MeCN ( 1 ·MeCN) and [Dy 2 ( hmi ) 2 (OAc) 2 (MeOH) 2 ]·H 2 O ( 2 ·H 2 O) with keto and enol forms of the corresponding ligands, respectively, were shown the similar core structures but different ratio of Dy III to OAc – . Moreover, the different coordination environments of complex [Dy 2 ( hb ) 2 (μ‐OAc) 2 (OAc) 2 (H 2 O) 2 ]·DMF·H 2 O ( 3 ·DMF·H 2 O) also offered an opportunity to understand the relationship between structural model and catalytic properties. Bimetallic dysprosium complexes 1 – 3 were demonstrated to be active catalysts for copolymerization of carbon dioxide (CO 2 ) and cyclohexene oxide (CHO) without cocatalysts. To the best of our knowledge, well‐defined catalyst 2 appears to be the first example of an air‐stable bimetallic dysprosium complex that is effective for CO 2 /CHO copolymerization and the formation of the perfectly alternating poly(cyclohexenecarbonate) with a high molecular weight. © 2016 Wiley Periodicals, Inc. J. Polym. Sci., Part A: Polym. Chem. 2017 , 55 , 321–328" @default.
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• W2535303503 date "2016-10-20" @default.
• W2535303503 modified "2023-10-18" @default.
• W2535303503 title "Copolymerization of carbon dioxide with cyclohexene oxide catalyzed by bimetallic dysprosium complexes containing hydrazine‐functionalized Schiff‐base derivatives" @default.
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• W2535303503 doi "https://doi.org/10.1002/pola.28387" @default.
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