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• W2536784013 abstract "Abstract High sensitive chemical sensors towards NO 2 and NH 3 based on the self‐assembled nanostructures of the heteroleptic and homoleptic bis(phthalocyaninato) europium complexes with octanaphthoxy phthalocyaninato ligands named Eu(Pc)[Pc(ONh) 8 ] ( 1 ) and Eu[Pc(ONh) 8 ] 2 ( 2 ) [Pc=unsubstituted phthalocyaninate; Pc(ONh) 8 =2,3,9,10,16,17,23,24‐octanaphthoxy phthalocyaninate] have been developed. The good conductivity, high crystallinity and large specific surface area for the self‐assemblies of 1 render it excellent sensing property for either electron‐accepting gas NO 2 in 50–250 ppb range or electron‐donating gas NH 3 in 2.5–12.5 ppm range due to the optimized molecular packing in the uniform‐sized nanoparticles depending on the effective intermolecular interaction between double‐decker molecules, among the best results of phthalocyanine‐based chemical sensors for detection of NO 2 and NH 3 at room temperature. Interestingly, self‐assemblies of 1 exhibited n ‐type response to NO 2 and p ‐type response to NH 3 , which is the first example of ambipolar charge‐transporting gas sensors fabricated from single‐component organic semiconductors. However, the self‐assemblies of 2 with sixteen bulky naphthoxy groups at the periphery of two Pc rings only present an n ‐type response to strong oxidant gas NO 2 in a relatively high concentration of 0.5–1.5 ppm, while are insensitive to weak reducing gas NH 3 due to the existence of great steric hindrance from bulky naphthoxy groups and more traps and/or defects in self‐assemblies." @default.
• W2536784013 created "2016-10-28" @default.
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• W2536784013 date "2016-10-01" @default.
• W2536784013 modified "2023-09-27" @default.
• W2536784013 title "High Sensitive Ambipolar Response towards Oxidizing NO₂ and Reducing NH₃ Based on Bis(phthalocyaninato) Europium Semiconductors" @default.
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• W2536784013 doi "https://doi.org/10.1002/cjoc.201600490" @default.
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