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• W2543284723 abstract "This study describes the use of polyisobutylene (PIB) to phase-anchor pyridine ligands that form a phase-separable Grubbs third-generation catalyst. We further show that this complex is useful in ring-opening metathesis polymerization (ROMP) reactions. These PIB-bound pyridine-ligated Grubbs catalysts provide the same benefits of control over polymer chain growth and polydispersity of the product as their low-molecular-weight analogs and reduce Ru leaching in ROMP products from approximately 16% (820 ppm residues) as seen with a similar pyridine-ligated catalyst to a value of approximately 3% (160 ppm residues). These labile ligands are shown to be as effective at generating separable metal complexes as less labile PIB-functionalized N-heterocyclic carbene catalyst ligands that are typically used for immobilization but that require a multistep synthesis." @default.
• W2543284723 created "2016-11-04" @default.
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• W2543284723 date "2016-10-27" @default.
• W2543284723 modified "2023-10-14" @default.
• W2543284723 title "Controlled Ring-Opening Metathesis Polymerization with Polyisobutylene-Bound Pyridine-Ligated Ru(II) Catalysts" @default.
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• W2543284723 doi "https://doi.org/10.1021/acsomega.6b00218" @default.
• W2543284723 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6640752" @default.
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