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• W2543363301 abstract "We report on the growth of a monolayer-thick ${mathrm{BiAg}}_{2}$ surface alloy on thin Ag films grown on Pt(111) and Cu(111). Using low energy electron diffraction (LEED), angle resolved photoemission spectroscopy (ARPES), and scanning tunneling microscopy (STM) we show that the surface structure of the $frac{1}{3}$ ML Bi/$x$-ML Ag/Pt(111) system ($xphantom{rule{4pt}{0ex}}ensuremath{ge}2$) is strongly affected by the annealing temperature required to form the alloy. As judged from the characteristic ($sqrt{3}ifmmodetimeselsetexttimesfi{}sqrt{3}$)$R{30}^{ensuremath{circ}}$ LEED pattern, the ${mathrm{BiAg}}_{2}$ alloy is partially formed at room temperature. A gentle, gradual increase in the annealing temperatures successively results in the formation of a pure ${mathrm{BiAg}}_{2}$ phase, a combination of that phase with a ($2ifmmodetimeselsetexttimesfi{}2$) superstructure, and finally the pure ($2ifmmodetimeselsetexttimesfi{}2$) phase, which persists at higher annealing temperatures. These results complement recent work reporting the ($2ifmmodetimeselsetexttimesfi{}2$) as a predominant phase, and attributing the absence of ${mathrm{BiAg}}_{2}$ alloy to the strained Ag/Pt interface. Likewise, we show that the growth of the ${mathrm{BiAg}}_{2}$ alloy on similarly lattice-mismatched 1 and 2 ML Ag-Cu(111) interfaces also requires a low annealing temperature, whilst higher temperatures result in ${mathrm{BiAg}}_{2}$ clustering and the formation of a ${mathrm{BiCu}}_{2}$ alloy. The demonstration that the ${mathrm{BiAg}}_{2}$ alloy can be formed on thin Ag films on different substrates presenting a strained interface has the prospect of serving as bases for technologically relevant systems, such as Rashba alloys interfaced with magnetic and semiconductor substrates." @default.
• W2543363301 created "2016-11-04" @default.
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• W2543363301 date "2016-10-28" @default.
• W2543363301 modified "2023-10-03" @default.
• W2543363301 title "Formation of the BiAg2 surface alloy on lattice-mismatched interfaces" @default.
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• W2543363301 doi "https://doi.org/10.1103/physrevb.94.155447" @default.
• W2543363301 hasPublicationYear "2016" @default.
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