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- W2543916322 endingPage "17799" @default.
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- W2543916322 abstract "Abstract The photoredox catalytic coupling of halomethyl arenes to bibenzyl derivatives has been demonstrated. The catalytic protocol employed the Hantzsch ester, potassium phosphate, and a photoactive cyclometalated Ir III complex catalyst. A photochemical quantum yield as high as 20 % was obtained. The catalytic mechanism was investigated in detail by performing photophysical and electrochemical measurements, as well as by quantum chemical calculations. The results suggest that two‐electron mediation might be responsible for the improved photon economy. The reaction protocol was compatible with halomethyl arenes that contain a variety of functional groups. Finally, the synthetic utility of our protocol was demonstrated by the preparation of a natural dihydrostilbenoid, brittonin A." @default.
- W2543916322 created "2016-11-04" @default.
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- W2543916322 creator A5024471296 @default.
- W2543916322 date "2016-10-28" @default.
- W2543916322 modified "2023-10-17" @default.
- W2543916322 title "Mechanism and Applications of the Photoredox Catalytic Coupling of Benzyl Bromides" @default.
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- W2543916322 doi "https://doi.org/10.1002/chem.201603517" @default.
- W2543916322 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27791290" @default.
- W2543916322 hasPublicationYear "2016" @default.
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