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- W2547069969 abstract "Abstract Four low symmetric A 2 B meso -substituted Cu(III)corroles with electron withdrawing meso -aryl rings have been synthesized and characterized. A detailed analysis of the optical and redox properties has been carried out by comparing their optical spectroscopy, electrochemistry and spectroelectrochemistry to a series of DFT and TD-DFT calculations. A series of experiments demonstrate that these Cu(III)corroles can be used as highly effective catalysts for hydrogen evolution reactions (HERs). Moreover, when the number of fluorine atoms at B meso -position is increased, there is a marked enhancement in the catalytic ability of the corrole complexes, which demonstrates that modification to the structures of low symmetry corroles is a useful strategy for developing new HER catalysts." @default.
- W2547069969 created "2016-11-11" @default.
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- W2547069969 date "2017-02-01" @default.
- W2547069969 modified "2023-09-24" @default.
- W2547069969 title "A2B type copper(III)corroles containing zero-to-five fluorine atoms: Synthesis, electronic structure and facile modulation of electrocatalyzed hydrogen evolution" @default.
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- W2547069969 doi "https://doi.org/10.1016/j.dyepig.2016.10.044" @default.
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