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- W2547801114 abstract "A Zn(II)−salicylaldimine complex [Zn(Lsalpyca)(H2O)]n (1, where H2Lsalpyca=4-hydroxy-3-(((pyridin-2-yl)methylimino)methyl)benzoic acid), with a one-dimensional (1D) chain structure, has been successfully converted to a discrete Ni(II)−salicylaldimine complex [Ni(Lsalpyca)(H2O)3] (2) and an infinite Cu(II)−salicylaldimine complex {[Cu(Lsalpyca)]·3H2O}n (3) through a metal-ion exchange induced structural transformation process. However, such processes do not worked by Mn(II) and Co(II) ions. Solid-state structure analyses reveal that complexes 1–3 form comparable coordinative or supramolecular zigzag chains running along the crystallographic [201] direction. In addition, replacing Zn(II) ion by Ni(II) and Cu(II) ions caused changes in coordination environment and sphere of metal centers, from a 5-coordinate intermediate geometry of square pyramidal and trigonal bipyramidal in 1 to a 6-coordinate octahedral geometry in 2, and to a 4-coordiante square planar geometry in 3. This study shows that metal-ion exchange serves as a very efficient way of forming new coordination complexes that may not be obtained through direct synthesis." @default.
- W2547801114 created "2016-11-11" @default.
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- W2547801114 date "2017-02-01" @default.
- W2547801114 modified "2023-09-27" @default.
- W2547801114 title "Metal-ion exchange induced structural transformation as a way of forming novel Ni(II)− and Cu(II)−salicylaldimine structures" @default.
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- W2547801114 doi "https://doi.org/10.1016/j.jssc.2016.10.026" @default.
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