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• W2550075177 endingPage "32476" @default.
• W2550075177 startingPage "32466" @default.
• W2550075177 abstract "Understanding the dynamics of electron-ion energy transfer in warm dense (WD) matter is important to the measurement of equation of state (EOS) properties and for understanding the energy balance in dynamic simulations. In this work, we present a comprehensive investigation of nonadiabatic electron relaxation and thermal excitation dynamics in aluminum under high pressure and temperature. Using quantum-classical trajectory surface hopping approaches, we examine the role of nonadiabatic couplings and electronic decoherence in electron-nuclear energy transfer in WD aluminum. The computed timescales range from 400 fs to 4.0 ps and are consistent with existing experimental studies. We have derived general scaling relationships between macroscopic parameters of WD systems such as temperature or mass density and the timescales of energy redistribution between quantum and classical degrees of freedom. The scaling laws are supported by computational results. We show that electronic decoherence plays essential role and can change the functional dependencies qualitatively. The established scaling relationships can be of use in modelling of WD matter." @default.
• W2550075177 created "2016-11-30" @default.
• W2550075177 creator A5062611755 @default.
• W2550075177 creator A5079911649 @default.
• W2550075177 creator A5083739979 @default.
• W2550075177 date "2016-01-01" @default.
• W2550075177 modified "2023-10-18" @default.
• W2550075177 title "Scaling relationships for nonadiabatic energy relaxation times in warm dense matter: toward understanding the equation of state" @default.
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• W2550075177 doi "https://doi.org/10.1039/c6cp06827h" @default.
• W2550075177 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27869257" @default.
• W2550075177 hasPublicationYear "2016" @default.
• W2550075177 type Work @default.

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