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- W2550454979 abstract "Abstract In order to correlate the physico-chemical properties of Ce x Zr 1-x O 2 catalysts with their catalytic activities for direct carboxylation of methanol to dimethyl carbonate (DMC), ceria-zirconia mixed oxides with the same nominal composition (Ce 0.5 Zr 0.5 O 2 ), which were prepared by different methods, were applied. The catalysts were characterized by means of XRD, N 2 adsorption, ICP-MS, NH 3 -TPD, CO 2 -TPD, Raman spectroscopy and XPS. Significant variations in their physico-chemical properties were observed by varying the preparation conditions. The results showed that the catalytic activity of the ceria-zirconia mixed oxides increased with improving the proportion of Ce 4+ , acidity and basicity of the catalyst surface. And the number of surface Ce 4+ content is the most important factor." @default.
- W2550454979 created "2016-11-30" @default.
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- W2550454979 date "2017-01-01" @default.
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- W2550454979 title "The proportion of Ce 4+ in surface of Ce x Zr 1-x O 2 catalysts: The key parameter for direct carboxylation of methanol to dimethyl carbonate" @default.
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- W2550454979 doi "https://doi.org/10.1016/j.jcou.2016.11.006" @default.
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