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• W2551386627 endingPage "035803" @default.
• W2551386627 startingPage "035803" @default.
• W2551386627 abstract "Rare-earth-doped ferromagnetic manganites La0.63RE0.07Sr0.30MnO3 (RE = Gd, Tb, Dy, and Ho) are synthesized in the form of sintered ceramics and nanocrystalline phases with the mean size of crystallites ≈30 nm. The electronic states of the dopants are investigated by SQUID magnetometry and theoretically interpreted based on the calculations of the crystal field splitting of rare-earth energy levels. The samples show the orthorhombic perovskite structure of Ibmm symmetry, with a complete FM order of Mn spins in bulk and reduced order in nanoparticles. Non-zero moments are also detected at the perovskite A sites, which can be attributed to magnetic polarization of the rare-earth dopants. The measurements in external field up to 70 kOe show a standard Curie-type contribution of the spin-only moments of Gd3+ ions, whereas Kramers ions Dy3+ and non-Kramers ions Ho3+ contribute by Ising moments due to their doublet ground states. The behaviour of non-Kramers ions Tb3+ is anomalous, pointing to singlet ground state with giant Van Vleck paramagnetism. The Tb3+ doping leads also to a notably increased coercivity compared to other La0.63RE0.07Sr0.30MnO3 systems." @default.
• W2551386627 created "2016-11-30" @default.
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• W2551386627 date "2016-11-16" @default.
• W2551386627 modified "2023-10-18" @default.
• W2551386627 title "Magnetic properties of rare-earth-doped La_0.7Sr_0.3MnO₃" @default.
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• W2551386627 doi "https://doi.org/10.1088/1361-648x/29/3/035803" @default.
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