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- W2551636713 abstract "Oxovanadium(IV), copper(II) and cobalt(II) acetylacetone complexes have been grafted onto amino-modified CMK-3-O (VO-NH2-CMK-3, Cu-NH2-CMK-3 and Co-NH2-CMK-3,respectively) and the materials thus prepared were used as heterogeneous catalysts for the aerobic oxidation of styrene. X-ray diffraction, nitrogen adsorption–desorption and transmission electron microscopy measurements confirmed the structural integrity of the mesoporous hosts, and spectroscopic characterization techniques (Fourier transform infrared, X-ray photoelectron, Raman) and thermogravimetry confirmed the ligands and the successful anchoring of the acetylacetone complexes to the modified mesoporous support. VO-NH2-CMK-3 displayed a relatively good catalytic performance with 94.6% of styrene conversion using air as oxidant, while Cu-NH2-CMK-3 gave 99.6% of styrene conversion using tert-butyl hydroperoxide as oxidant. Copyright © 2015 John Wiley & Sons, Ltd." @default.
- W2551636713 created "2016-11-30" @default.
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- W2551636713 date "2015-08-06" @default.
- W2551636713 modified "2023-09-25" @default.
- W2551636713 title "Oxovanadium(IV), copper(II) or cobalt(II) acetylacetone complexes immobilized on amino-functionalized CMK-3 for the aerobic epoxidation of styrene" @default.
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- W2551636713 doi "https://doi.org/10.1002/aoc.3353" @default.
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