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- W2552490410 abstract "An enantioselective, copper-catalyzed alkynylation of cyclic α,α-diaryl ketiminium ions has been developed to deliver isoquinoline products with diaryl, tetrasubstituted stereocenters. The success of this reaction relied on identification of Ph-PyBox as the optimal ligand, i-Pr2NEt as the base, and CHCl3 as the solvent. A broad scope and functional group tolerance were observed. Notably, the use of both aryl and silyl acetylenes results in high yields and enantioselectivities. Mechanistic experiments are consistent with a dimeric or higher order catalyst." @default.
- W2552490410 created "2016-11-30" @default.
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- W2552490410 date "2016-11-16" @default.
- W2552490410 modified "2023-10-16" @default.
- W2552490410 title "Enantioselective, Copper-Catalyzed Alkynylation of Ketimines To Deliver Isoquinolines with α-Diaryl Tetrasubstituted Stereocenters" @default.
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- W2552490410 doi "https://doi.org/10.1021/acs.orglett.6b02787" @default.
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