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• W2553614483 abstract "Abstract A Pd-YSZ cermet membrane that performs coupled operations of hydrogen separation from a mixed-gas stream and simultaneous hydrogen production by non-galvanic water-splitting, and have high sulfur tolerance is fabricated. It is proved that in H 2 S containing atmosphere the Pd-YSZ membrane has self-repairing capability, originating mainly from the conversion of Pd 4 S back to metallic Pd and SO 2 by ambipolar-diffused oxygen obtained from water-splitting. The performance of membrane was analyzed at different temperatures in high H 2 S containing (0–4000 ppm H 2 S) mixed gas feed during the operation as a hydrogen separation membrane as well as during the coupled operation of hydrogen separation and hydrogen production. At 900 °C with the feed-stream having ≥2000 ppm H 2 S, the hydrogen flux was severely affected due to the formation of some liquid phase of Pd 4 S, resulting in the segregation of hydrogen permeating Pd-phase at the membrane surface. But at 800 °C, though the membrane was affected by the Pd 4 S formation in high H 2 S environment (up to 1200 ppm H 2 S), its self-repairing capability and additional hydrogen production by water-splitting is capable of maintaining the hydrogen flux around ~1.24 cm 3 (STP)/min.cm 2 , a value expected by the same membrane while performing only the hydrogen separation function in H 2 S-free environment." @default.
• W2553614483 created "2016-11-30" @default.
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• W2553614483 date "2017-02-01" @default.
• W2553614483 modified "2023-09-23" @default.
• W2553614483 title "Pd-YSZ cermet membranes with self-repairing capability in extreme H2S conditions" @default.
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• W2553614483 doi "https://doi.org/10.1016/j.ceramint.2016.11.011" @default.
• W2553614483 hasPublicationYear "2017" @default.
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