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• W2554485859 abstract "A square-planar Co4 amide cluster, Co4{N(SiMe3)2}4 (2), and an octahedral Co6 hydride cluster, Co6H8(PiPr3)6 (4), were obtained from metathesis-type amide to hydride exchange reactions of a CoII amide complex with pinacolborane (HBpin) in the absence/presence of PiPr3. The crystal structure of 4 revealed face-capping hydrides on each triangular [Co3] face, while the formal CoII2CoI4 oxidation state of 4 indicated a reduction of the cobalt centers during the assembly process. Cluster 4 catalyzes the hydrosilylation of 2-cyclohexen-1-one favoring the conjugate reduction. Generation of the catalytically reactive Co cluster species was indicated by a trapping experiment with a chiral chelating agent." @default.
• W2554485859 created "2016-11-30" @default.
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• W2554485859 date "2016-11-16" @default.
• W2554485859 modified "2023-10-16" @default.
• W2554485859 title "Co₆H₈(P^<i>i</i>Pr₃)₆: A Cobalt Octahedron with Face-Capping Hydrides" @default.
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• W2554485859 doi "https://doi.org/10.1002/anie.201608262" @default.
• W2554485859 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27862749" @default.
• W2554485859 hasPublicationYear "2016" @default.
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