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• W2555033260 endingPage "672" @default.
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• W2555033260 abstract "A novel quinone-modified metal-organic frameworks NH2-MIL-101(Fe) was synthesized using a simple chemical method under mild condition. The introduced 2-anthraquinone sulfonate (AQS) can be covalently modified with NH2-MIL-101(Fe) and acts as a redox mediator to enhance the degradation of bisphenol A (BPA) via persulfate activation. The obtained AQS-NH-MIL-101(Fe) was characterized by Fourier transform infrared spectroscopy, X-ray diffraction, scanning electron microscopy, X-ray photoelectron spectra, cyclic voltammetry and electrochemical impedance spectroscopy. AQS-NH-MIL-101(Fe) exhibited better catalytic performance compared with NH2-MIL-101(Fe) and NH2-MIL-101(Fe) with free AQS (NH2-MIL-101(Fe)/AQS). That is, AQS-NH-MIL-101(Fe) was proved to be the most effective in that more than 97.7% of BPA was removed. The degradation rate constants (k) of AQS-NH-MIL-101(Fe) was 9-fold higher than that of NH2-MIL-101(Fe) and 7-fold higher than NH2-MIL-101(Fe)/AQS, indicating that AQS is a great electron-transfer mediator when modified with NH2-MIL-101(Fe). Based on the above results, the possible mechanism of catalytic reaction has been investigated in view of the trapping experiments. In addition, the AQS-NH-MIL-101(Fe) catalyst exhibited excellent stability and can be used several times without significant deterioration in performance." @default.
• W2555033260 created "2016-11-30" @default.
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• W2555033260 date "2017-02-01" @default.
• W2555033260 modified "2023-10-16" @default.
• W2555033260 title "Quinone-modified NH2-MIL-101(Fe) composite as a redox mediator for improved degradation of bisphenol A" @default.
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• W2555033260 doi "https://doi.org/10.1016/j.jhazmat.2016.11.040" @default.
• W2555033260 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/27876243" @default.
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