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• W2556304032 abstract "Liquid-liquid transition is an intriguing phenomenon in which a liquid transforms into another liquid via the first-order transition. For molecular liquids, however, it always takes place in a supercooled liquid state metastable against crystallization, which has led to a number of serious debates concerning its origin: liquid-liquid transition vs. unusual nano-crystal formation. Thus, there have so far been no single example free from such debates. Here we show the first firm experimental evidence that the transition is truly liquid-liquid transition and not nano-crystallization for a molecular liquid, triphenyl phosphite. We kinetically isolate the reverse liquid-liquid transition from glass transition and crystallization with an extremely high heating rate of flash differential scanning calorimetry, and prove the reversibility and first-order nature of liquid-liquid transition. Our finding not only deepens our physical understanding of liquid-liquid transition but also will initiate a new phase of its research from both fundamental and applications viewpoints." @default.
• W2556304032 created "2016-11-30" @default.
• W2556304032 creator A5005967783 @default.
• W2556304032 creator A5077985868 @default.
• W2556304032 date "2016-11-14" @default.
• W2556304032 modified "2023-10-13" @default.
• W2556304032 title "The reversibility and first-order nature of liquid–liquid transition in a molecular liquid" @default.
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• W2556304032 doi "https://doi.org/10.1038/ncomms13438" @default.
• W2556304032 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5114579" @default.
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• W2556304032 hasPublicationYear "2016" @default.
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