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- W2557673870 abstract "We measured the optical transitions due to the internal energy levels of an exciton and biexciton in a CuCl single crystal using pump-probe spectroscopy. The transient absorption bands due to the transitions from the $1s$ to $2p$ and from the $1s$ to $3p$ exciton states were observed at 3 K, which is consistent with their reported energies. Simultaneously, the transient absorption peak due to the biexciton was observed, which corresponds to a transition from the lowest state (composed of two $1s$ excitons) to higher states (composed of $1s$ and $2p$ excitons). The value of the observed biexciton peak energy was reasonable considering the hydrogen molecule orbitals and the electron-to-hole effective mass ratio. In addition, the transient absorption peaks were broadened at 77 K, because of the increase in the homogeneous width of the $2p$ exciton state. The transient absorption spectrum was almost completely determined by this width. Our findings are of importance with regard to the optical phenomena in the infrared region related to the quantum coherence of excitons and biexcitons in semiconductors." @default.
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- W2557673870 date "2016-11-28" @default.
- W2557673870 modified "2023-09-24" @default.
- W2557673870 title "Optical transitions from the lowest to higher exciton and biexciton Rydberg states in CuCl" @default.
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- W2557673870 doi "https://doi.org/10.1103/physrevb.94.195209" @default.
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