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• W2559674448 abstract "Abstract The ever-growing demand for environmentally friendly and efficient energy systems has stimulated significant efforts for the design of advanced electroactive fabrics. This paper reports facile control over heterogeneous mesoarchitectures of N-Co3O4@C unit blocks oriented along the c-axis arch. Three basic types of nanoscale architectures, namely, nanorod pellets (NRPs), nanoneedles (NNs), and crossed-X nanosheets (X-NSs), can be built in a vertical fashion along the c-axis orientations. The atomic structures of the developed N-Co3O4@C-NRP, NN, and X-NS catalysts were dominant along the dense exposure {1 1 2} plane, low-index crystal {0 0 1}, and {1 1 1} facets, respectively. Among all the nanoscale architectures, the NRPs revealed superior methanol oxidation reaction (MOR) in terms of oxidation current and onset potential, indicating the key role of the top-Co3+ sites along the dense exposure crystal {1 1 2} facet. Results indicate that the heterogeneous N-Co3O4@C-NRP catalyst showed efficient electrochemical reactions and better long-term stability than commercial Pt/C catalyst." @default.
• W2559674448 created "2016-12-08" @default.
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• W2559674448 date "2017-04-01" @default.
• W2559674448 modified "2023-10-18" @default.
• W2559674448 title "Axially oriented tubercle vein and X-crossed sheet of N-Co3O4@C hierarchical mesoarchitectures as potential heterogeneous catalysts for methanol oxidation reaction" @default.
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• W2559674448 doi "https://doi.org/10.1016/j.cej.2016.12.003" @default.
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