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- W2559955944 abstract "In this thesis, photoinduced SCO dynamics of single crystal Fe(PM-AzA)2](NCS)2 is studied by DC-RF hybrid femtosecond electron diffraction system (FED). The temporal characteristics of the high brightness electron pulses is characterized by a photo-triggered streak camera. The results of the FED experiment show that the structural changes of the metal and ligand and electronic state changes in the metal atom are concomitant but not simultaneous. The metal-ligand bond elongation, compared to other nuclear motions in the photoinduced SCO, is not a conclusive signature of the photoinduced SCO, and it is coupled to the other nuclear motions in phase transition. The metal-ligand bond elongation (and other nuclear motions) is significantly delayed with respect to the electronic SCO transitions. In dieser Arbeit wird photoinduzierte SCO-Dynamik von Monokristall Fe(PM-AzA)2](NCS)2) durch die DC-RF-Hybrid-FED untersucht . Die zeitlichen Eigenschaften der Elektronenpulse mit hohen Helligkeit wird von einem photoinduzierten Streak-Kamera gemessen. Die Ergebnisse des FED-Experiments zeigen, dass die Strukturanderungen des Metalls und Ligands und die elektronische Zustandsanderungen in dem Metallatom sind begleitend, aber nicht gleichzeitig. Die Dehnung einer Metall-Ligand-Bindung, im Vergleich zu anderen Kernbewegungen in der photoinduzierten SCO, ist kein ausschlaggebender Faktor des photoinduziertes SCO. Sie wird mit den anderen Kernbewegungen in Phasenubergang kombiniert. Die Dehnung einer Metall-Ligand-Bindung (und andere Kernbewegungen) ist, im Vergleich zu SCO-Dynamiken, signifikant verzogert." @default.
- W2559955944 created "2016-12-16" @default.
- W2559955944 creator A5044136716 @default.
- W2559955944 date "2016-12-01" @default.
- W2559955944 modified "2023-09-24" @default.
- W2559955944 title "Femtosecond Electron diffraction Studies of Photoinduced Spin Crossover in Single Crystal [Fe(PM-AzA)2](NCS)2" @default.
- W2559955944 hasPublicationYear "2016" @default.
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