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- W2560128453 abstract "Donor–acceptor cyclopropanes were engaged in a [3+3]-annulation reaction with γ-hydroxyenones. Sc(OTf)3 was found to be the best catalyst, and 2,4,4,5-tetrasubstituted tetrahydropyran products were obtained in good yields under mild reaction conditions. The generality of the reaction permitted the synthesis of tetrasubstituted tetrahydropyrans bearing aryl, alkyl, and heteroaromatic groups. A catalytic asymmetric variant of this process was also studied preliminary with a chiral PyBOX ligand." @default.
- W2560128453 created "2016-12-16" @default.
- W2560128453 creator A5020812219 @default.
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- W2560128453 date "2017-01-18" @default.
- W2560128453 modified "2023-09-26" @default.
- W2560128453 title "Lewis Acid Catalyzed [3+3] Annulation of Donor-Acceptor Cyclopropanes with γ-Hydroxyenones: Access to Highly Functionalized Tetrahydropyrans" @default.
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- W2560128453 doi "https://doi.org/10.1002/ejoc.201601305" @default.
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