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• W2560134441 abstract "A series of a novel beryllium-free KBBF family of nonlinear-optical materials AZn2BO3X2 (A = K, Rb and X = Cl; A = Na, K, Rb and X = Br) were successfully synthesized through molecular engineering design, and single crystals of AZn2BO3Cl2 (A = K, Rb) were grown by a spontaneous nucleation technique from self-flux systems. As a representative for the halogen KBBF family of crystals, KZn2BO3Cl2 features the infinite lattice layer [Zn2BO3Cl2]∞ made up of BO3 and ZnO3Cl anionic groups, and the in-layer BO3 groups are completely coplanar and well-aligned. Besides, KZn2BO3Cl2 exhibits high transmittance in the range of 300-2000 nm with a UV-transmission cutoff of around 200 nm according to transmission spectra. The compounds of AZn2BO3Cl2 (A = K, Rb) are both phase-matchable with powder second-harmonic-generation efficiencies of 1.3 and 1.17 times that of KH2PO4 for KZn2BO3Cl2 and RbZn2BO3Cl2, respectively, which are similar to that of KBBF." @default.
• W2560134441 created "2016-12-16" @default.
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• W2560134441 date "2016-12-07" @default.
• W2560134441 modified "2023-10-17" @default.
• W2560134441 title "Beryllium-Free KBBF Family of Nonlinear-Optical Crystals: AZn₂BO₃X₂ (A = Na, K, Rb; X = Cl, Br)" @default.
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• W2560134441 doi "https://doi.org/10.1021/acs.inorgchem.6b02044" @default.
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