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- W2562096043 abstract "Hydrogen storage is an important aspect to enable the so-called hydrogen economy. Mg-Ni alloys are among the most promising candidates for solid-state hydrogen storage systems yet many questions remain unanswered regarding the hydriding/dehydriding mechanism of the alloys. Mg2NiH4 particularly has received much attention both for its potential as a hydrogen storage medium and also exhibits interesting properties relating to its different polymorphs. Here, the dehydriding mechanism in bulk Mg2NiH4 is investigated using in-situ ultra-high voltage transmission electron microscopy (TEM) combined with Synchrotron powder X-ray diffraction (XRPD) and differential scanning calorimetry (DSC). We find that the hydrogen release is based on a mechanism of nucleation and growth of Mg2NiHx (x∼0–0.3) solid solution grains and is greatly enhanced in the presence of crystal defects occurring as a result of the polymorphic phase transformation. Also importantly, with atomic resolution TEM imaging a high density of stacking faults is identified in the dehydrided Mg2NiHx (x∼0–0.3) lattices." @default.
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- W2562096043 date "2017-02-01" @default.
- W2562096043 modified "2023-10-06" @default.
- W2562096043 title "In-situ investigation of the hydrogen release mechanism in bulk Mg2NiH4" @default.
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- W2562096043 doi "https://doi.org/10.1016/j.jpowsour.2016.11.105" @default.
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