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- W2562962007 abstract "The reactivity and the regioselective functionalization of silyl–diene enol ethers under a bifunctional organocatalyst provokes a dramatic change in the regioselectivity, from the 1,5- to the 1,3-functionalization. This variation makes possible the 1,3-addition of silyl–dienol ethers to nitroalkenes, giving access to the synthesis of tri- and tetrasubstituted double bonds in Rauhut–Currier type products. The process takes place under smooth conditions, nonanionic conditions, and with a high enantiomeric excess. A rational mechanistic pathway is presented based on DFT and mechanistic experiments." @default.
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- W2562962007 date "2017-01-09" @default.
- W2562962007 modified "2023-10-17" @default.
- W2562962007 title "Asymmetric Synthesis of Rauhut–Currier type Products by a Regioselective Mukaiyama Reaction under Bifunctional Catalysis" @default.
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- W2562962007 doi "https://doi.org/10.1021/jacs.6b07851" @default.
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