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• W2564037646 abstract "The surface structures, high-voltage charging/discharging performances, and Li-ion transfer at the electrode/electrolyte interface of LiNi1/3Co1/3Mn1/3O2 coated with small amounts of Zr oxide by the sol-gel method were investigated. Island-like ZrO2 grains as well as grain-free (sea-like) zones were observed on the surfaces of the coated LiNi1/3Co1/3Mn1/3O2 samples. The ratio of the area of these sea-like zones to the total surface area of the LiNi1/3Co1/3Mn1/3O2 sample increased from 44 to 85% when the Zr oxide content was decreased from 1.0 to 0.125 wt%. A compound oxide phase containing Zr, Ni, Co, and Mn was formed uniformly on the sea-like zones; the depth of this phase was approximately 2 nm. The initial discharge capacities of the coated LiNi1/3Co1/3Mn1/3O2 samples were equal to that of bare LiNi1/3Co1/3Mn1/3O2. Further, the cycling performances of the coated LiNi1/3Co1/3Mn1/3O2 samples were significantly higher, as were their discharge capacities and discharge voltages, while their charge-transfer resistances (Rct) were lower. It was also found that the coated LiNi1/3Co1/3Mn1/3O2 samples had lower activation energies (Ea) for charge transfer than the bare LiNi1/3Co1/3Mn1/3O2. Thus, it can be surmised that the area and structure of the sea-like zones determined the Rct and Ea values and cycling performances of the coated LiNi1/3Co1/3Mn1/3O2 samples." @default.
• W2564037646 created "2017-01-06" @default.
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• W2564037646 date "2015-11-05" @default.
• W2564037646 modified "2023-10-16" @default.
• W2564037646 title "Surface Structure and High-Voltage Charging/Discharging Performance of Low-Content Zr-Oxide-Coated LiNi_1/3Co_1/3Mn_1/3O₂" @default.
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• W2564037646 doi "https://doi.org/10.1149/2.0211602jes" @default.
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