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- W2564728049 abstract "This paper reports the synthesis of hierarchical aluminosilicate inorganic polymers (also known as geopolymers) containing both Bronsted and Lewis acid sites that function as a new class of heterogeneous solid acid catalysts. The geopolymers were synthesised from a naturally occurring clay mineral by an energy-efficiently and ecologically friendly process. Their catalytic performance was evaluated in a model liquid phase Friedel-Crafts alkylation of relatively large substituted benzenes (alkylation of toluene, anisole, p-xylene and mesitylene with benzyl chloride). The influence of the geopolymer starting composition on the acidity and porosity of the synthesised catalysts was studied and the impact of post-synthetic demetallation on their catalytic performance was investigated. The geopolymer-based catalysts achieved high catalytic activity which was superior to HY zeolite under identical reaction conditions. These results suggest that geopolymers have considerable potential as cost efficient, readily synthesised and environmentally friendly heterogeneous solid catalysts for fine chemical applications." @default.
- W2564728049 created "2017-01-06" @default.
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- W2564728049 date "2017-03-01" @default.
- W2564728049 modified "2023-10-14" @default.
- W2564728049 title "Facile synthesis of new hierarchical aluminosilicate inorganic polymer solid acids and their catalytic performance in alkylation reactions" @default.
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- W2564728049 doi "https://doi.org/10.1016/j.micromeso.2016.12.018" @default.
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