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- W2564804530 abstract "Abstract SO 3 -Ph-BTBP is a hydrophilic tetra-N-dentate ligand proposed for An(III)/Ln(III) separation by solvent extraction, and a candidate for use in future advanced reprocessing schemes such as GANEX and SANEX. We present the first study of the effect of SO 3 -Ph-BTBP on the corrosion behavior of stainless steels. Specifically, studies have been performed using steels and conditions equivalent to those found in relevant nuclear reprocessing flow sheets. SO 3 -Ph-BTBP has been shown to have little effect on either steel passivation or reductive dissolution. However, if driven cathodically into a region of hydrogen evolution at the electrode surface or conversely anodically into a region of transpassive dissolution, observed currents are reduced in the presence of SO 3 -Ph-BTBP, suggesting corrosion inhibition of the steel potentially through weak absorption of a SO 3 -Ph-BTBP layer at the metal-solution interface. The lack of any observed corrosion acceleration via complexation of Fe 3+ is surprising and has been suggested to be due to the slow extraction kinetics of SO 3 -Ph-BTBP as a result of a requirement for a trans- to cis-conformational change before binding." @default.
- W2564804530 created "2017-01-06" @default.
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- W2564804530 date "2015-12-01" @default.
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- W2564804530 title "The effect of SO3-Ph-BTBP on stainless steel corrosion in nitric acid" @default.
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- W2564804530 doi "https://doi.org/10.1515/nuka-2015-0117" @default.
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