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- W2565432992 abstract "We synthesized the novel $S=1/2{mathrm{Mo}}_{3}$ cluster magnet ${mathrm{Li}}_{2}{mathrm{ScMo}}_{3}{mathrm{O}}_{8}$ as well as the isomorphic compound ${mathrm{Li}}_{2}{mathrm{InMo}}_{3}{mathrm{O}}_{8}$, and investigated their macroscopic and microscopic physical properties. ${mathrm{Li}}_{2}{mathrm{InMo}}_{3}{mathrm{O}}_{8}$ showed magnetic ordering at ${T}_{N}ensuremath{sim}12$ K with a ${120}^{ensuremath{circ}}$ structure, while no magnetic ordering is observed down to 0.5 K in ${mathrm{Li}}_{2}{mathrm{ScMo}}_{3}{mathrm{O}}_{8}$ despite the strong antiferromagnetic interaction among clusters probed by the Weiss temperature. Results of the $^{7}mathrm{Li}$ nuclear magnetic resonance spectra and the nuclear spin-lattice relaxation rate $(1/{T}_{1})$ measurement show direct microscopic proof of the spin-disordered ground state. We discuss the difference in the ground state between ${mathrm{Li}}_{2}{mathrm{ScMo}}_{3}{mathrm{O}}_{8}$ and ${mathrm{Li}}_{2}{mathrm{InMo}}_{3}{mathrm{O}}_{8}$ using the description of localized magnetism based on spin frustration within the triangular lattice and that of inter- and intracluster charge fluctuations." @default.
- W2565432992 created "2017-01-06" @default.
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- W2565432992 date "2015-07-09" @default.
- W2565432992 modified "2023-09-23" @default.
- W2565432992 title "Spin-liquid behavior in the spin-frustrated<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mi>Mo</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:math>cluster magnet<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:msub><mml:mi>Li</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi>ScMo</mml:mi><mml:mn>3</mml:mn></mml:msub><mml:msub><mml:mi mathvariant=normal>O</mml:mi><mml:mn>8</mml:mn></mml:msub></mml:mrow></mml:math>in contrast to magnetic …" @default.
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- W2565432992 doi "https://doi.org/10.1103/physrevb.92.014409" @default.
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