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• W2567394584 abstract "A mononuclear complex, [LCo(L′)2]ClO4⋅MeOH⋅H2O (1) (L′=4-aminopyridine) and a binuclear heterometallic complex, [LCo(L′′)2Na(ClO4)2]⋅0.5H2O (2) (L′′=1-methylimidazole) have been prepared from a Schiff-base ligand (H2L=N, N′-bis(3-methoxysalicylidehydene)cyclohexane-1,2-diamine). The formation of both complexes were confirmed by employing several analytical techniques including single crystal X-ray diffraction. The molecular structure of 1 consists of a [LCo(L′)2]+ cation associated with a [ClO4]− ion. Complex 2 contains a Co(III) ion and a Na(I) ion and thus it results a heterometallic Co(III)-Na(I) compound. The Co(III) ion is in a distorted octahedral geometry in both complexes. Phenoxazinone synthase activity of 1 and 2 have been investigated. The oxidation of 2-aminophenol (OAPH) to 2-aminophenoxazine-3-one (APX) follows saturation rate kinetics with the formation of a catalyst-substrate adduct. Mass analysis and electrochemical properties of both complexes have been investigated and they are in full support of the saturation rate kinetics." @default.
• W2567394584 created "2017-01-06" @default.
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• W2567394584 date "2016-12-16" @default.
• W2567394584 modified "2023-09-27" @default.
• W2567394584 title "Syntheses, Structures and Phenoxazinone Synthase Activities of Two Cobalt(III) Complexes" @default.
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• W2567394584 doi "https://doi.org/10.1002/slct.201601597" @default.
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