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• W2567609669 abstract "Molecular photoswitches incorporated in a junction present a way to achieve light-controlled conductance switching by photoisomerization. Yet, the two isomers might also interconvert upon charging of the molecule if this results in a change in their relative energies. This behavior (current-induced switching) has been termed dark photoswitching and was observed for the dihydroazulene–vinylheptafulvene couple in a junction. In this theoretical study, we expand this concept to dimeric structures containing two dihydroazulene units linked through meta- or para-phenylene bridges and anchored to the electrodes through different linkers. In particular, we show how stepwise dark photoswitching can be achieved for certain redox states." @default.
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• W2567609669 date "2017-02-02" @default.
• W2567609669 modified "2023-09-23" @default.
• W2567609669 title "Stepwise “Dark Photoswitching” of Photochromic Dimers in a Junction" @default.
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• W2567609669 doi "https://doi.org/10.1021/acs.jpcc.6b10410" @default.
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