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- W2567749087 abstract "Abstract Field-effect transistors (FETs) based on solution-processed indium-gallium-zinc oxide (IGZO) exhibited excellent electrical properties, including a high carrier mobility over 1 cm 2 /V s and an on/off current ratio over 10 7 . Solution-processable gate dielectric materials with excellent electrical strength were required instead of inorganic oxide gate dielectrics such as SiO 2 , Al 2 O 3 , and HfO 2 . In this manuscript, we demonstrated the use of a ladder-type poly(phenyl- co -methacryl silsesquioxane) (PPMSQ) copolymer as a gate dielectric in IGZO FETs. Methacryloxypropyl groups in the copolymer were introduced to crosslink the polymer chains via thermal annealing. Thermal annealing at 200 °C enhanced the electrical strength of the gate dielectric layer because of the formation of a network structure with a reduced free volume. The resulting IGZO FETs based on 200 °C-annealed ladder-type PPMSQ gate dielectrics exhibited an electron mobility of 1.2 (±0.05) cm 2 /V s, a threshold voltage of 17 (±2) V, and an on/off current ratio of 1.5 (±0.7) × 10 8 . The use of the polymeric ladder-type PPMSQ gate dielectrics for gating the IGZO FETs provided a novel approach to realizing future flexible electronics." @default.
- W2567749087 created "2017-01-13" @default.
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- W2567749087 date "2017-04-01" @default.
- W2567749087 modified "2023-10-16" @default.
- W2567749087 title "Ladder-type silsesquioxane copolymer gate dielectrics for gating solution-processed IGZO field-effect transistors" @default.
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- W2567749087 doi "https://doi.org/10.1016/j.orgel.2017.01.009" @default.
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