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- W2567935753 abstract "Elucidating the intrinsic water wettability of the graphitic surface has increasingly attracted research interests, triggered by the recent finding that the well-established hydrophobicity of graphitic surfaces actually results from airborne hydrocarbon contamination. Currently, static water contact angle (WCA) is often used to characterize the intrinsic water wettability of graphitic surfaces. In the current paper, we show that because of the existence of defects, static WCA does not necessarily characterize the intrinsic water wettability. Freshly exfoliated graphite of varying qualities, characterized using atomic force microscopy and Raman spectroscopy, was studied using static, advancing, and receding WCA measurements. The results showed that graphite of different qualities (i.e., defect density) always has a similar advancing WCA, but it could have very different static and receding WCAs. This finding indicates that defects play an important role in contact angle measurements, and the static contact angle does not always represent the intrinsic water wettability of pristine graphite. On the basis of the experimental results, a qualitative model is proposed to explain the effect of defects on static, advancing, and receding contact angles. The model suggests that the advancing WCA reflects the intrinsic water wettability of pristine (defect-free) graphite. Our results showed that the advancing WCA for pristine graphite is 68.6°, which indicates that graphitic carbon is intrinsically mildly hydrophilic." @default.
- W2567935753 created "2017-01-13" @default.
- W2567935753 creator A5025182962 @default.
- W2567935753 creator A5059246379 @default.
- W2567935753 creator A5075889094 @default.
- W2567935753 creator A5089710232 @default.
- W2567935753 date "2017-01-20" @default.
- W2567935753 modified "2023-09-24" @default.
- W2567935753 title "Characterization of the Intrinsic Water Wettability of Graphite Using Contact Angle Measurements: Effect of Defects on Static and Dynamic Contact Angles" @default.
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- W2567935753 doi "https://doi.org/10.1021/acs.langmuir.6b04193" @default.
- W2567935753 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28071919" @default.
- W2567935753 hasPublicationYear "2017" @default.
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