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- W2570290710 abstract "Abstract Coal tar is one of the valuable chemical materials and energy, from which the nitrogen-containing compounds ( N -compounds), indole, carbazole, pyridine, and quinoline, are mainly separated. In the present work, the imidazolium-based ILs with different anions, 1-butyl-3-methyl-imidazolium chloride (BmimCl), 1-butyl-3-methyl-imidazolium bromide (BmimBr), 1-butyl-3-methyl-imidazolium tetrafluoroborate (BmimBF 4 ), 1-butyl-3-methyl-imidazolium disulfate (BmimHSO 4 ), and 1-butyl-3-methyl-imidazolium acetate (BmimCH 3 COO), were used to separate those N -compounds via extraction. The performances of ILs extraction were evaluated by the extraction efficiency and distribution coefficient. High extraction efficiency and selectivity could be found for the neutral N -compounds, indole and carbazole, by BmimCl than basic N -compounds, pyridine and quinoline. Meanwhile, the optimized conditions were ascertained and the selected ILs could be easily regenerated by water and be sustainable recycled by a back-extraction process. Furthermore, a hydrogen bond was formed between the neutral N -compound and the selected ILs, and the mechanism was confirmed based on the analysis by a molecular simulation. Thus, an approach was provided for the separation of neutral N -compounds from coal tar." @default.
- W2570290710 created "2017-01-13" @default.
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- W2570290710 date "2017-04-01" @default.
- W2570290710 modified "2023-10-18" @default.
- W2570290710 title "Extraction and mechanism for the separation of neutral N -compounds from coal tar by ionic liquids" @default.
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- W2570290710 doi "https://doi.org/10.1016/j.fuel.2016.12.095" @default.
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