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- W2570613845 abstract "Significance Uranium is an important fuel source and pollutant, and its chemical form determines its reactivity in the environment. However, information on the speciation of tetravalent U [U(IV)] in sediments is lacking. The research presented herein takes a holistic view of U(IV) speciation in a natural material containing microbial cells, organic matter, and minerals. Our work demonstrates unequivocally that U(IV) adsorbs to natural organic matter under anoxic, field-relevant conditions. Furthermore, we put forward a conceptual model that provides a framework for future studies of U biogeochemistry in which postreduction surface complexation processes can be used to predict U(IV) behavior. Our work has ramifications for remediation of U-contaminated sites and also informs in situ mining practices." @default.
- W2570613845 created "2017-01-13" @default.
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- W2570613845 date "2017-01-09" @default.
- W2570613845 modified "2023-10-16" @default.
- W2570613845 title "Uranium(IV) adsorption by natural organic matter in anoxic sediments" @default.
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- W2570613845 doi "https://doi.org/10.1073/pnas.1611918114" @default.
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