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• W2575057869 abstract "Architectural control over the mesoporous TiO2 film, a common electron-transport layer for organic-inorganic hybrid perovskite solar cells, is conducted by employing sub-micron sized polystyrene beads as sacrificial template. Such tailored TiO2 layer is shown to induce asymmetric enhancement of light absorption notably in the long-wavelength region with red-shifted absorption onset of perovskite, leading to ~20% increase of photocurrent and ~10% increase of power conversion efficiency. This enhancement is likely to be originated from the enlarged CH3NH3PbI3(Cl) grains residing in the sub-micron pores rather than from the effect of reduced perovskite-TiO2 interfacial area, which is supported from optical bandgap change, haze transmission of incident light, and one-diode model parameters correlated with the internal surface area of microporous TiO2 layers. With the templating strategy suggested, the necessity of proper hole-blocking method is discussed to prevent any direct contact of the large perovskite grains infiltrated into the intended pores of TiO2 scaffold, further mitigating the interfacial recombination and leading to ~20% improvement in power conversion efficiency compared with the control device using conventional solution-processed hole blocking TiO2. Thereby, the imperatives that originate from the structural engineering of the electron-transport layer are discussed to understand the governing elements for the improved device performance." @default.
• W2575057869 created "2017-01-26" @default.
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• W2575057869 date "2017-01-19" @default.
• W2575057869 modified "2023-09-25" @default.
• W2575057869 title "Tailoring the Mesoscopic TiO2 Layer: Concomitant Parameters for Enabling High-Performance Perovskite Solar Cells" @default.
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• W2575057869 doi "https://doi.org/10.1186/s11671-016-1809-7" @default.
• W2575057869 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5247386" @default.
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