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• W2575389640 abstract "Despite the fact that carbon dioxide is an abundant atmospheric gas with profound environmental implications, there is little information on the reaction of carbon dioxide at the adsorbed water−oxide interface. In this study, the chemistry of carbon dioxide at the adsorbed water−iron oxide interface is investigated with FTIR spectroscopy. As shown here, the thin water layer on the iron oxide surface plays an important role in the surface chemistry of carbon dioxide. In particular, adsorbed water enhances CO2 uptake, undergoes isotope exchange with CO2 in O(18)-labeled experiments, and influences the chemical nature of the predominant adsorbed product on the surface from bicarbonate to carbonate. The resultant thin water film is acidic in nature from the reaction of CO2. The IR spectrum recorded of adsorbed carbonate at the adsorbed water−iron oxide interface is remarkably similar to that at the bulk liquid water−iron oxide interface. Since reactions in thin water films estimated to be ∼2 layers will play a role in a number of environmental processes, it is essential to understand the chemistry of these “wet” interfaces with atmospheric gases." @default.
• W2575389640 created "2017-01-26" @default.
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• W2575389640 date "2005-06-01" @default.
• W2575389640 modified "2023-09-25" @default.
• W2575389640 title "Surface Reactions of Carbon Dioxide at the Adsorbed Water−Iron Oxide Interface" @default.
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• W2575389640 doi "https://doi.org/10.1021/jp051868k" @default.
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