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- W2575694515 abstract "Abstract A palladium‐catalyzed aminopalladation reaction followed by nucleophilic addition with aldehydes and dehydration is described. This direct and operationally simple procedure provides a rapid and reliable approach to a wide range of functionalized tetrahydroisoquinolines with high selectivity. Mechanistic studies disclosed that the nucleophilic addition, performed via a highly ordered transition‐state, is the turnover‐limiting step in which the inherent β‐hydride elimination of the key Csp 3 −Pd species was controlled by the confined conformation and the nucleophilicity of the Csp 3 −Pd bond was enhanced by the strong electron‐donating effect of the nitrogen atom." @default.
- W2575694515 created "2017-01-26" @default.
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- W2575694515 date "2017-01-20" @default.
- W2575694515 modified "2023-10-08" @default.
- W2575694515 title "Palladium-Catalyzed Ring-Forming Aminoalkenylation of Alkenes with Aldehydes Initiated by Intramolecular Aminopalladation" @default.
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- W2575694515 doi "https://doi.org/10.1002/anie.201611853" @default.
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