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- W257770923 abstract "Author(s): Martin, Rhia Marissa | Advisor(s): Bergman, Robert G | Abstract: Recently in the Ellman and Bergman groups a method was discovered for preparing 1,2-dihydropyridines via rhodium-catalyzed coupling of α,β-unsaturated imines and alkynes. Subsequent in situ oxidation provides access to the corresponding pyridines. This method was expanded to include terminal alkynes, challenging substrates for transition-metal mediated transformations. In contrast formal reduction of the dihydropyridine intermediates through Diels-Alder reaction with alkenes provides access to isoquinuclidines, an important class of piperidines, in excellent diastereoselectivities." @default.
- W257770923 created "2016-06-24" @default.
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- W257770923 date "2012-01-01" @default.
- W257770923 modified "2023-09-27" @default.
- W257770923 title "Synthesis of Pharmaceutically Relevant Nitrogen Heterocycles via Rhodium Catalyzed C-H Bond Functionalization" @default.
- W257770923 hasPublicationYear "2012" @default.
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