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- W2577793481 abstract "We have carried out a comparative study of plausible non-180° domain configurations in the two- and three-phase states of lead-free ferroelectrics Ba(Ti1−x Zr x )O3 (0.02 ≤ x ≤ 0.08) and (Ba0.85Ca0.15)(Ti0.90Zr0.10)O3, respectively, using the elastic matching approach. The phase contents and stress-relief conditions in Ba(Ti0.93Zr0.07)O3 and (Ba0.85Ca0.15)(Ti0.90Zr0.10)O3 strongly depend on domain types in the rhombohedral R3m phase, whereas domains of the orthorhombic Amm2 phase influence two-phase states in Ba(Ti0.98Zr0.02)O3. Changes in unit-cell parameters of (Ba0.85Ca0.15)(Ti0.90Zr0.10)O3 at poling lead to the complete stress relief in three-phase (P4mm + Amm2 + R3m) structures by increasing the volume fraction of the R3m phase. A link between the heterophase/domain structures and high piezoelectric activity in (Ba0.85Ca0.15)(Ti0.90Zr0.10)O3 is discussed. Based on our results, we state that equal or almost equal volume fractions of the domain types at the three-phase coexistence in (Ba0.85Ca0.15). .(Ti0.90Zr0.10)O3 can lead to an enhanced contribution from domain-wall displacements and therefore, to the large piezoelectric response in this important lead-free ferroelectric compound." @default.
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- W2577793481 date "2017-01-18" @default.
- W2577793481 modified "2023-09-24" @default.
- W2577793481 title "Plausible domain configurations and phase contents in two- and three-phase BaTiO<sub>3</sub>-based lead-free ferroelectrics" @default.
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- W2577793481 doi "https://doi.org/10.1088/1361-6463/aa51ae" @default.
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