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• W2577865864 abstract "Examples of coordination compounds in which KrF2 functions as a ligand are very rare. In contrast, XeF2 provides a rich coordination chemistry with a variety of main-group and transition metal cations. The reactions of Mg(AsF6 )2 and KrF2 in HF or BrF5 solvent have afforded [Mg(KrF2 )4 (AsF6 )2 ] and [Mg(KrF2 )4 (AsF6 )2 ]⋅2 BrF5 , respectively, the first examples of a metal cation ligated by KrF2 . Their X-ray crystal structures and Raman spectra show that the KrF2 ligands and [AsF6 ]- anions are F-coordinated to a naked Mg2+ cation. Quantum-chemical calculations are consistent with essentially non-covalent ligand-metal bonding. These compounds significantly extend the XeF2 -KrF2 analogy and the limited chemistry of krypton by introducing a new class of coordination compound in which KrF2 functions as a ligand towards a naked metal cation." @default.
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• W2577865864 date "2017-01-12" @default.
• W2577865864 modified "2023-10-17" @default.
• W2577865864 title "Coordination of KrF₂ to a Naked Metal Cation, Mg²⁺" @default.
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• W2577865864 doi "https://doi.org/10.1002/anie.201611534" @default.
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