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• W2579962384 abstract "In this work, we compare the intensity ratio of symmetric to antisymmetric CO stretching vibrational transitions in CO2− and MCOO− (M = H, Ag and Bi) using photodissociation spectroscopy. We observe that this ratio depends strongly on the bonding partner M. We trace this behavior to a dynamic change in the charge distribution of the molecules during vibrational motion by comparing the derivatives of the dipole moment during vibrational motion calculated from a fixed-charge approximation, a charge distribution analysis, and the prediction of the infrared spectra of the ions under study. The calculations are based on density functional theory." @default.
• W2579962384 created "2017-02-03" @default.
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• W2579962384 date "2017-09-01" @default.
• W2579962384 modified "2023-09-23" @default.
• W2579962384 title "Enhancement of infrared activity by moving electrons through bonds – The case of CO2 anion and carboxylate" @default.
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• W2579962384 doi "https://doi.org/10.1016/j.cplett.2017.01.060" @default.
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