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• W2580452089 endingPage "3266" @default.
• W2580452089 startingPage "3262" @default.
• W2580452089 abstract "Understanding the fundamental processes taking place on Co surfaces during the Fischer–Tropsch (FT) synthesis is of great interest and importance. We herein report a self-anticoking mechanism of a cobalt surface by subsurface oxygen. The active carbidic carbon species for FT synthesis tends to transform into the inactive graphitic carbon species on clean Co(0001) and poisons the Co surface. Subsurface atomic oxygen on Co(0001) can stabilize the active carbidic carbon species and quench the transformation process. These results reveal, to the best of our knowledge, for the first time the reactivity of various surface species on Co surfaces that dynamically maintain a delicate balance to enhance the long-term stability of Co catalysts during FT synthesis." @default.
• W2580452089 created "2017-02-03" @default.
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• W2580452089 date "2017-02-14" @default.
• W2580452089 modified "2023-10-05" @default.
• W2580452089 title "Self-Anticoking of a Cobalt Surface by Subsurface Oxygen in the Fischer-Tropsch Synthesis" @default.
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• W2580452089 doi "https://doi.org/10.1002/chem.201605577" @default.
• W2580452089 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28116798" @default.
• W2580452089 hasPublicationYear "2017" @default.
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