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• W2581080883 abstract "We performed a study of the single ionization of iodine, ${mathrm{I}}_{2}$ over a range of wavelengths. Single ionization of ${mathrm{I}}_{2}$ is unexpectedly found to have a contribution from inner molecular orbitals involving the $5s$ electrons. The $text{I}+{text{I}}^{+}$ dissociation channel was recorded through velocity map imaging, and the kinetic-energy release of each channel was determined with two-dimensional fitting of the images. Most of the measured kinetic-energy data were inconsistent with ionization to the $X, A$, and $B$ states of ${mathrm{I}}_{2}{}^{+}$, implying ionization from deeper orbitals. A pump-probe Fourier transform technique was used to look for modulation at the $X$- and $A$-state vibrational frequencies to see if they were intermediate states in a two-step process. $X$- and $A$-state modulation was seen only for kinetic-energy releases below 0.2 eV, consistent with dissociation through the $B$ state. From these results and intensity-, polarization-, and wavelength-dependent experiments we found no evidence of bond softening, electron rescattering, or photon mediation through the $X$ or $A$ states to higher-energy single-ionization channels." @default.
• W2581080883 created "2017-02-03" @default.
• W2581080883 creator A5001810730 @default.
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• W2581080883 date "2017-01-24" @default.
• W2581080883 modified "2023-09-24" @default.
• W2581080883 title "Single ionization of molecular iodine" @default.
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• W2581080883 doi "https://doi.org/10.1103/physreva.95.013410" @default.
• W2581080883 hasPublicationYear "2017" @default.
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