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• W2590933468 abstract "Molybdenum-99 is the parent of the most widely used medical isotope technetium-99m. Proliferation concerns have prompted development of alternative Mo production methods utilizing low enriched uranium. Alumina and titania sorbents were evaluated for separation of Mo from concentrated uranyl nitrate solutions. System, mass transfer, and isotherm parameters were determined to enable design of Mo separation processes under a wide range of conditions. A model-based approach was utilized to design representative commercial-scale column processes. The designs and parameters were verified with bench-scale experiments. The results are essential for design of Mo separation processes from irradiated uranium solutions, selection of support material, and process optimization. Mo uptake studies show that adsorption decreases with increasing concentration of uranyl nitrate; however, examination of Mo adsorption as a function of nitrate ion concentration shows no dependency, indicating that uranium competes with Mo for ..." @default.
• W2590933468 created "2017-03-03" @default.
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• W2590933468 date "2017-03-06" @default.
• W2590933468 modified "2023-10-12" @default.
• W2590933468 title "Design of a Fission ⁹⁹Mo Recovery Process and Implications toward Mo Adsorption Mechanism on Titania and Alumina Sorbents" @default.
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• W2590933468 doi "https://doi.org/10.1021/acs.iecr.6b04667" @default.
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