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- W2592897765 abstract "A series of isoreticular metal–organic frameworks (MOFs) of the formula M(BDC)(L) (M = Fe(II) or Co(II), BDC = 1,4-benzenedicarboxylate, L = pyrazine (pyz) or 4,4′-bipyridine (bipy)) has been synthesized and characterized by N2 gas uptake measurements, single crystal and powder X-ray diffraction, magnetometry, X-ray absorption spectroscopy, and Mössbauer spectroscopy. These studies indicate the formation of a permanently porous solid with high-spin Fe(II) and Co(II) centers that are weakly coupled, consistent with first-principles density functional theory calculations. This family of materials represents unusual examples of paramagnetic metal centers coordinated by linkers capable of mediating magnetic or electronic coupling in a porous framework. While only weak interactions are observed, the rigid 3D framework of the MOF dramatically impacts the properties of these materials when compared with close structural analogues." @default.
- W2592897765 created "2017-03-16" @default.
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- W2592897765 date "2017-03-03" @default.
- W2592897765 modified "2023-10-17" @default.
- W2592897765 title "Incorporation of Pyrazine and Bipyridine Linkers with High-Spin Fe(II) and Co(II) in a Metal–Organic Framework" @default.
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- W2592897765 doi "https://doi.org/10.1021/acs.inorgchem.6b02883" @default.
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