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- W2593155141 abstract "We report on the low-temperature scanning tunneling microscopy (STM) measurements of the self-assembly of nonplanar 10,10'-dibromo-9,9'-bianthryl (DBBA) molecules on Ag(111) combined with density functional theory (DFT) calculations. DBBA molecules have two enantiomorphous adsorption configurations, from which more chiral structures can be formed. At a low coverage [0.4 monolayer (ML)], DBBA forms racemic netlike islands consisting of molecular chains along ⟨1 2 3̅⟩Ag. Moreover, the gliding between the molecular chains gives rise to chiral windmill-like patterns in the islands. At 0.8 ML, DBBA forms a racemic row phase and a homochiral hexamer phase. The molecular appearance difference between the two coexisted phases and the DFT calculated molecular adsorption configuration reveal a decrease in the molecular dihedral angle of DBBA, which implies an enhancement in the intermolecular interactions via CH···π and halogen bonds. The transition from a racemic packing mode to a homochiral one suggests that the suitability of steric configurations is dominant in the close-packing mode under enhanced intermolecular interactions." @default.
- W2593155141 created "2017-03-16" @default.
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- W2593155141 date "2017-03-15" @default.
- W2593155141 modified "2023-10-17" @default.
- W2593155141 title "Chiral Self-Assembly of Nonplanar 10,10′-Dibromo-9,9′-bianthryl Molecules on Ag(111)" @default.
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- W2593155141 doi "https://doi.org/10.1021/acs.langmuir.7b00218" @default.
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