Matches in SemOpenAlex for { <https://semopenalex.org/work/W2593882466> ?p ?o ?g. }
- W2593882466 endingPage "3732" @default.
- W2593882466 startingPage "3726" @default.
- W2593882466 abstract "We use analytical theory and numerical simulation to study the role of short-range hydrodynamics (lubrication forces) in determining the lifetime of colloidal bonds. Such insight is useful in understanding many aspects of colloidal systems, such as gelation, nucleation, yielding, and rejuvenation, and as a paradigm for diffusion-controlled dissociation reactions in liquids. Our model system consists of spherical particles with an attractive square-well potential of variable width δ. We find that the predicted colloidal bond lifetimes can be substantially increased upon the inclusion of lubrication forces, to an extent that depends on the attraction range. An analytical law is derived that predicts this enhancement as a function of the well width, in quantitative agreement with simulation data. For sufficiently short-ranged attraction, lubrication forces dramatically enhance the drag on two bonded particles, leading to reduced effective diffusion coefficients and, hence, longer bond lifetimes. This effect disappears upon an increase in the width of the attractive wells beyond a length scale comparable to the particle diameter. The simulation further suggests that the role of lubrication forces becomes less important as confinement is increased, i.e., upon approaching the supersaturation limit, ϕ ≈ 0.5, where caging effects become important. Our findings complement recent studies of the role of long-range hydrodynamic interactions, contributing to a comprehensive description of the subtle link between hydrodynamics and bonding in attractive colloids." @default.
- W2593882466 created "2017-03-16" @default.
- W2593882466 creator A5077414687 @default.
- W2593882466 creator A5087484656 @default.
- W2593882466 date "2017-03-24" @default.
- W2593882466 modified "2023-10-03" @default.
- W2593882466 title "Effect of Hydrodynamic Interactions on the Lifetime of Colloidal Bonds" @default.
- W2593882466 cites W1925483670 @default.
- W2593882466 cites W1963972730 @default.
- W2593882466 cites W1964489076 @default.
- W2593882466 cites W1967734745 @default.
- W2593882466 cites W1969287097 @default.
- W2593882466 cites W1985746657 @default.
- W2593882466 cites W1989925383 @default.
- W2593882466 cites W2002754781 @default.
- W2593882466 cites W2004857915 @default.
- W2593882466 cites W2005661781 @default.
- W2593882466 cites W2006340321 @default.
- W2593882466 cites W2019465613 @default.
- W2593882466 cites W2020869169 @default.
- W2593882466 cites W2025672520 @default.
- W2593882466 cites W2047953352 @default.
- W2593882466 cites W2052664100 @default.
- W2593882466 cites W2066295790 @default.
- W2593882466 cites W2072968302 @default.
- W2593882466 cites W2076741768 @default.
- W2593882466 cites W2085266415 @default.
- W2593882466 cites W2087145339 @default.
- W2593882466 cites W2091293700 @default.
- W2593882466 cites W2092144432 @default.
- W2593882466 cites W2093365639 @default.
- W2593882466 cites W2097333170 @default.
- W2593882466 cites W2116689416 @default.
- W2593882466 cites W2128899338 @default.
- W2593882466 cites W2146510553 @default.
- W2593882466 cites W2157001218 @default.
- W2593882466 cites W2171007695 @default.
- W2593882466 cites W2329849883 @default.
- W2593882466 cites W2335889050 @default.
- W2593882466 cites W2472630932 @default.
- W2593882466 cites W2491403440 @default.
- W2593882466 cites W2950027670 @default.
- W2593882466 cites W3101592052 @default.
- W2593882466 cites W3104501523 @default.
- W2593882466 cites W3106042146 @default.
- W2593882466 doi "https://doi.org/10.1021/acs.iecr.7b00337" @default.
- W2593882466 hasPublicationYear "2017" @default.
- W2593882466 type Work @default.
- W2593882466 sameAs 2593882466 @default.
- W2593882466 citedByCount "9" @default.
- W2593882466 countsByYear W25938824662018 @default.
- W2593882466 countsByYear W25938824662019 @default.
- W2593882466 countsByYear W25938824662020 @default.
- W2593882466 countsByYear W25938824662021 @default.
- W2593882466 countsByYear W25938824662023 @default.
- W2593882466 crossrefType "journal-article" @default.
- W2593882466 hasAuthorship W2593882466A5077414687 @default.
- W2593882466 hasAuthorship W2593882466A5087484656 @default.
- W2593882466 hasBestOaLocation W25938824662 @default.
- W2593882466 hasConcept C102931765 @default.
- W2593882466 hasConcept C111368507 @default.
- W2593882466 hasConcept C121332964 @default.
- W2593882466 hasConcept C127313418 @default.
- W2593882466 hasConcept C147789679 @default.
- W2593882466 hasConcept C159467904 @default.
- W2593882466 hasConcept C159985019 @default.
- W2593882466 hasConcept C184608416 @default.
- W2593882466 hasConcept C185592680 @default.
- W2593882466 hasConcept C192562407 @default.
- W2593882466 hasConcept C200447597 @default.
- W2593882466 hasConcept C204323151 @default.
- W2593882466 hasConcept C2778517922 @default.
- W2593882466 hasConcept C57879066 @default.
- W2593882466 hasConcept C59789625 @default.
- W2593882466 hasConcept C61048295 @default.
- W2593882466 hasConcept C69357855 @default.
- W2593882466 hasConcept C72921944 @default.
- W2593882466 hasConcept C97355855 @default.
- W2593882466 hasConceptScore W2593882466C102931765 @default.
- W2593882466 hasConceptScore W2593882466C111368507 @default.
- W2593882466 hasConceptScore W2593882466C121332964 @default.
- W2593882466 hasConceptScore W2593882466C127313418 @default.
- W2593882466 hasConceptScore W2593882466C147789679 @default.
- W2593882466 hasConceptScore W2593882466C159467904 @default.
- W2593882466 hasConceptScore W2593882466C159985019 @default.
- W2593882466 hasConceptScore W2593882466C184608416 @default.
- W2593882466 hasConceptScore W2593882466C185592680 @default.
- W2593882466 hasConceptScore W2593882466C192562407 @default.
- W2593882466 hasConceptScore W2593882466C200447597 @default.
- W2593882466 hasConceptScore W2593882466C204323151 @default.
- W2593882466 hasConceptScore W2593882466C2778517922 @default.
- W2593882466 hasConceptScore W2593882466C57879066 @default.
- W2593882466 hasConceptScore W2593882466C59789625 @default.
- W2593882466 hasConceptScore W2593882466C61048295 @default.
- W2593882466 hasConceptScore W2593882466C69357855 @default.
- W2593882466 hasConceptScore W2593882466C72921944 @default.
- W2593882466 hasConceptScore W2593882466C97355855 @default.
- W2593882466 hasFunder F4320334903 @default.